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Increase max_children to 150 and restart fpm. Also, check the php-fpm error log. It should have further clues on why it’s failing.
It’s happening because your max_connections is being reached. Run these commands and copy/paste the output here:
wget http://mysqltuner.pl
mv index.html mysqltuner.pl
perl mysqltuner.pl
On the last command, you might need to run it like this:
perl mysqltuner.pl --user root -pass <mysql_root_passwd>
I had the same issue and solved it by adding a SWAP to my droplet following “How To Add Swap Space on Ubuntu 20.04”